If I'm understanding what you are wanting; increase the number of cores/threads reserved for the GPU and limit the CPU tasks from interfering with GPU tasks, then the answer is to use ProLasso. With that program you can assign both priority and affinity for each executable regardless of what BOINC tries to do. For example, I could be running 8 CPU tasks (BOINC scheduler) and have them run on 4 threads of the processor.
So, figure of argument, you want to reserve 4 threads for the CPU and 4 threads for the GPU, you would "right" click on the CPU executable name and then select "affinity". Then assign the threads the CPU can use. Then right click on the GPU executable name and assign the threads for the GPU. You can also select the "priority" (this really does matter big time). Since the CPU tasks and GPU tasks won't be using the same cores you can set them both up to "above normal". The benefit to using ProLasso is that the GPU tasks and CPU tasks aren't using the same cores and having to do a memory swap every time it wants to service the executable.
You only have to make the affinity/priority setting one time and ProLasso remembers your setting for that executable. In the future if you change your GPU tasks and don't need as many threads reserved then you can right click on the CPU executable and give it more threads.
If you decide to use this on an 8 thread machine, then if you have reserved 4 threads for the CPU then you should set BOINC "use processors" so that it is using 50% PLUS (GPU default cpu requirement * number of instances). ie the GPU (from project) request .5 cpu and you are running 4 instances simultaneously then you would set BOINC PROCESSORS to 4 + 2 (6) so the BOINC scheduler would run 4 CPU tasks. Obviously, with affinity set the CPU tasks won't interfere with the GPU, but if running 6 instances of the CPU on 4 threads then the CPU tasks become less efficient since it is doing memory swap every time it services an executable.
It isn't as difficult as my description sounds ... it is intuitively obvious once you install and take a look at ProLasso.
ProLasso is free for 30 days and then some of the features go away. HOWEVER, the stuff you care about (affinity and priority) are always available!